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Phys. Rev. A 80, 033817 (2009) [10 pages]

Theoretical and experimental analysis of quantum path interferences in high-order harmonic generation

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T. Auguste* and P. Salières
CEA–Saclay, IRAMIS, Service des Photons, Atomes et Molécules, F-91191 Gif-sur-Yvette, France

A. S. Wyatt, A. Monmayrant, and I. A. Walmsley
Clarendon Laboratory, Parks Road, Oxford OX1 3PU, United Kingdom

E. Cormier
CELIA, CNRS-CEA–Université Bordeaux 1, 351 Cours de la Libération, 33405 Talence, France

A. Zaïr, M. Holler, A. Guandalini, F. Schapper, J. Biegert§, L. Gallmann, and U. Keller
Physics Department, ETH Zurich, CH-8093 Zurich, Switzerland

Received 7 May 2009; published 10 September 2009

See accompanying Physics Synopsis

We present theoretical and experimental studies on quantum path interferences in high-order harmonic generation. Simulations of the single-atom response allow us to calculate the different quantum paths contributions; their relative phases and the resulting interferences can be finely controlled through the laser intensity that provides an efficient means for controlling the electron trajectories with an accuracy on the ten attoseconds time scale. Simulations of the macroscopic response demonstrate the need of spatial and spectral filtering of the harmonic beam in order to observe the interferences between the two shortest quantum paths. Our numerical results are in very good agreement with experimental data. These investigations represent a step toward the full characterization and control of the atomic harmonic dipole.

© 2009 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevA.80.033817
DOI:
10.1103/PhysRevA.80.033817
PACS:
42.65.Ky, 32.80.Rm

*Corresponding author; thierry.auguste@cea.fr

Present address: LAAS-CNRS, 31077 Toulouse, France.

Present address: Department of Physics, Blackett Laboratory, Imperial College London, South Kensington Campus, London SW7 2BW, UK.

§Present address: ICFO, 08860 Castelldefels (Barcelona), Spain.