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Phys. Rev. A 79, 053814 (2009) [5 pages]

Laser-field-related recombination interference in high-order harmonic generation from CO2 molecules

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Pengfei Wei1, Peng Liu1, Jing Chen2, Zhinan Zeng1, Xiaodong Guo1, Xiaochun Ge1, Ruxin Li1,*, and Zhizhan Xu1,†
1State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
2Institute of Applied Physics and Computational Mathematics, P.O. Box 8009, Beijing 100088, People’s Republic of China

Received 18 November 2008; published 7 May 2009

We reinvestigate the modulation inversion of angular distribution of high-order harmonic generation (HHG) from impulsively aligned CO2 molecules. The angular distribution is found to be sensitive to both the harmonic order and the intensity of the driving laser pulse for HHG. The roles of intramolecular quantum interference and the laser intensity are clarified. A laser-field-related recombination interference model is proposed to explain the modulation inversion of harmonic yield with respect to the molecular alignment. We conclude that the two-center interference in the recombination process can be manipulated by changing the laser intensity.

© 2009 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevA.79.053814
DOI:
10.1103/PhysRevA.79.053814
PACS:
42.65.Ky, 42.65.Re

*ruxinli@mail.shcnc.ac.cn

zzxu@mail.shcnc.ac.cn