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Phys. Rev. A 79, 041201(R) (2009) [4 pages]

Ionization and charge migration through strong internal fields in clusters exposed to intense x-ray pulses

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Christian Gnodtke, Ulf Saalmann, and Jan M. Rost
Max Planck Institute for the Physics of Complex Systems, Nöthnitzer Straße 38, 01187 Dresden, Germany and Max Planck Advanced Study Group at the Center for Free-Electron Laser Science, Luruper Chaussee 149, 22761 Hamburg, Germany

Received 11 December 2008; published 27 April 2009

A general scenario for electronic charge migration in finite samples illuminated by an intense laser pulse is given. Microscopic calculations for neon clusters under strong short pulses as produced by x-ray free-electron laser sources confirm this scenario and point to the prominent role of field ionization by strong internal fields. The latter leads to the fast formation of a core-shell system with an almost static core of screened ions while the outer shell explodes. Substituting the shell ions with a different material such as helium as a sacrificial layer leads to a substantial improvement of the diffraction image for the embedded cluster thus reducing the consequences of radiation damage for coherent diffractive imaging.

© 2009 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevA.79.041201
DOI:
10.1103/PhysRevA.79.041201
PACS:
36.40.Wa, 87.59.−e, 87.15.ht, 41.60.Cr