Multiorder coherent Raman scattering of a quantum probe field

We study the multiorder coherent Raman scattering of a quantum probe field in a far-off-resonance medium with a prepared coherence. Under the conditions of negligible dispersion and limited bandwidth, we derive a Bessel-function solution for the sideband field operators. We analytically and numerically calculate various quantum statistical characteristics of the sideband fields. We show that the multiorder coherent Raman process can replicate the statistical properties of a single-mode quantum probe field into a broad comb of generated Raman sidebands. We also study the mixing and modulation of photon statistical properties in the case of two-mode input. We show that the prepared Raman coherence and the medium length can be used as control parameters to switch a sideband field from one type of photon statistics to another type, or from a nonsqueezed state to a squeezed state and vice versa. We demonstrate that an even or odd coherent state of the quantum probe field can produce a multipartite entangled coherent state. We show that the concurrence reaches its maximal value at an optimal medium length that is determined by the magnitude of the Raman coherence and the orders of the Raman sidebands.