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Phys. Rev. A 66, 033205 (2002) [7 pages]

Energy transfer in collisions of metal clusters with multiply charged ions

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J. Daligault1,2, F. Chandezon1,*, C. Guet1,3, B. A. Huber1,4, and S. Tomita1,5
1Département de Recherche Fondamentale sur la Matière Condensée, CEA-Grenoble, 17, rue des Martyrs, F-38054 Grenoble Cedex 9, France
2Los Alamos National Laboratory, Theoretical Division, MS-K 717, Los Alamos, New Mexico 87545
3Département de Physique Théorique et Appliquée, CEA-DAM-Ile de France, Boîte Postale 12, F-91680 Bruyères-le-Chatel, France
4CIRIL-GANIL, Rue Claude Bloch, Boîte Postale 5133, F-14070 Caen Cedex 05, France
5Institute of Physics and Astronomy, University of Aarhus, DK-8000 Aarhus C, Denmark

Received 22 April 2002; published 27 September 2002

Collisions between low-energy multiply charged ions and neutral metal clusters are an efficient method to investigate charge instabilities in finite systems. We study here the appearance size napp(q) of multiply charged sodium clusters Nanq+ with q<~10, i.e., the smallest size of observation for q-fold charged clusters and its dependence on the collision parameters. The experimental results are compared with the energy transferred to the cluster during the collision, calculated with the semiclassical Vlasov equation within the jellium approximation. Experimental and theoretical data show similar trends with the collision parameters and evidence the importance of dynamical effects. These results guide further investigations for studying low excited multiply charged finite systems.

© 2002 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevA.66.033205
DOI:
10.1103/PhysRevA.66.033205
PACS:
36.40.Qv, 31.15.Gy, 34.50.Gb

*Email address: fchandezon@cea.fr