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Phys. Rev. A 58, 3942–3952 (1998)

Single- and multiple-electron dynamics in the strong-field tunneling limit

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B. Sheehy, R. Lafon, M. Widmer, B. Walker*, and L. F. DiMauro
Chemistry Department, Brookhaven National Laboratory, Upton, New York 11973

P. A. Agostini
Service des Photons, Atomes et Molecules, Centre d’Etudes de Saclay, 91191 Gif Sur Yvette, France

K. C. Kulander
Theoretical Atomic and Molecular Physics Group, Lawrence Livermore National Laboratory, Livermore, California 94551

Received 18 March 1998; published in the issue dated November 1998

Evolution of atomic ionization into the strong-field limit offers the opportunity to study the fundamentals of atom-laser interaction. In this study, we report on high precision measurements of the ion and electron distributions from laser-excited helium and neon atoms which reflect the changing continuum dynamics as the ionization process evolves into the pure tunneling regime. The experiments present evidence of both single- and two-electron ionization. These data provide a direct quantitative test of various theories of strong-field ionization. We show that a relatively simple semiclassical model which includes a description of a field-driven electron elastically rescattering from an accurate ion core potential reproduces the measured electron distributions for both atoms. However, using this model to calculate e-2e inelastic rescattering yields cross sections which are incompatible with the measured two-electron ionization.

© 1998 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevA.58.3942
DOI:
10.1103/PhysRevA.58.3942
PACS:
32.80.Rm, 31.90.+s, 32.80.Fb

*Present address: Dept. of Chemistry, University of California, San Diego, LaJolla, CA 92093.